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Carbon nanotube (CNT) and graphene are the most popular materials being studied currently since they carry on so many significant features which are unbelievable to normal materials. By re-designing and decorating the micro-structure, they demonstrate an even greater flexibility to meet human needs. Raman technology is a good tool to collect RBM spectra in CNT and G-band/ D-band in graphene due to the fact that the small Raman peak shift is proof right from the slightly different structure, making it an ideal instrument to characterize the material structure in carbon science.